† Corresponding author. E-mail:
Project supported by the National Natural Science Foundation of China (Grant Nos. 11647122 and 61705064) and the Natural Science Foundation of Hubei Province, China (Grant Nos. 2018CFB672 and 2018CFB773).
An ultrafast and low-power slow light tuning mechanism based on plasmon-induced transparency (PIT) for two disk cavities aperture-coupled to a metal-dielectric-metal plasmonic waveguide system is investigated numerically and analytically. The optical Kerr effect is enhanced by the local electromagnetic field of surface plasmon polaritons, slow light, and graphene–Ag composite material structures with a large effective Kerr nonlinear coefficient. Through the dynamic adjustment of the frequency of the disk nanocavity, the group velocity is controlled between c/53.2 and c/15.1 with the pump light intensity increased from 0.41 MW/cm2 to 2.05 MW/cm2. Alternatively, through the dynamic adjustment of the propagation phase of the plasmonic waveguide, the group velocity is controlled between c/2.8 and c/14.8 with the pump light intensity increased from 5.88 MW/cm2 to 11.76 MW/cm2. The phase shift multiplication of the PIT effect is observed. Calculation results indicate that the entire structure is ultracompact and has a footprint of less than 0.8 μm2. An ultrafast responsive time in the order of 1 ps is reached due to the ultrafast carrier relaxation dynamics of graphene. All findings are comprehensively analyzed through finite-difference time-domain simulations and with a coupling-mode equation system. The results can serve as a reference for the design and fabrication of nanoscale integration photonic devices with low power consumption and ultrafast nonlinear responses.
Slow light is a crucial element in the study of quantum information processing, optical communication, and all-optical storage. The effective realization of slow light depends on the development of electromagnetically induced transparency (EIT). Quantum destructive interference between the excitation pathways to the atomic upper level indicates that the peculiar and counter-intuitive phenomenon called EIT has appeared in the atomic system.[1] EIT performance in transparent windows with strong dispersion and enhanced transmitted characteristics[2] indicates that EIT can be widely used in enhanced optical nonlinearity, optical data storage, and sensors. The potential application of the EIT effect is obstructed by its requirements of extreme cold environments and stable gas lasers. Nevertheless, researchers have demonstrated that plasmon-induced transparency (PIT) can be obtained in photonic nanostructures.[3] The PIT effect is similar to the classical EIT and has attracted extensive attention due to its potential for use in information-processing chips and integrated photonic devices.[4] The PIT effect causes a strong destructive interference between narrowband dark and wideband bright patterns.[5] As a particular case of Fano resonance, the PIT effect with steep dispersion decreases the group velocity.[6] The enhancement capability is large in accordance with the local electromagnetic (EM) field, and the typical diffraction limit caused by surface plasmon polaritons (SPPs) is solved; thus, a device based on the PIT effect can be used with a small footprint.[7] The PIT effects on plasmonic nanostructures have been demonstrated in many schemes, such as metamaterials,[8–14] graphene structures,[15–20] metal nanowire grating-coupled dielectric waveguides,[21] and metal photonic crystals.[22] The metal–dielectric–metal (MDM) plasmonic waveguide side-coupling cavity has elicited widespread attention because it can achieve on-chip PIT effects.[23–26] In addition, plasmonic waveguide side-coupling cavity structures can be easily fabricated on integrated photonic chips. However, researchers have rarely studied slow light in MDM plasmonic waveguide platforms by using aperture-coupled disk resonators.
Conventional realization of PIT effect and slow light is achieved by adjusting the structural parameters of plasmonic nanostructures, such as the metal damping factor, resonator diameter, and coupling distance.[4] Once the geometric parameters of these nanostructures are confirmed, the majority of plasmonic-coupled systems cannot actively control the PIT effect. As a static system, this type of nanostructure is limited by the bandwidth–delay product. The operating bandwidth is conversely proportional to the maximal accomplishable group delay.[27] This limitation of the bandwidth–delay product can be overcome through the dynamic adjustment of the PIT effect and slow light in a coupled nanocavity system. However, achieving ultrafast and low-power dynamically adjustable PIT effects and slow light on the nanophotonic devices remain challenging.
Many integrated photonic devices need a dynamically adjustable PIT effect and slow light, that is, the peak wavelength, the size of the PIT window, and the group index change with the structure parameters. Yang et al. reported an on-chip adjustable PIT effect in four plasmonic comb cavities coupled waveguide system. The cavities were overlaid by a 100 nm thick poly(methy1 methacrylate) (PMMA) layer.[28] The response time of PMMA was in the microsecond range. Therefore, the third-order nonlinear Kerr effect was used to realize subpicosecond or even femtosecond ultrafast response time. In addition, Lu et al. and Pu et al. researched resonators and MDM waveguides full of nonlinear Kerr material Ag-BaO.[29,30] On the basis of the considerably small third-order nonlinear susceptibility of the traditional optical Kerr material, the threshold pump light intensity can be as high as 1 GW/cm2. For dynamically adjustable slow light, the conventional implementation method involves adjusting the propagation phase of the plasmonic waveguide in a coupled waveguide system or using radiative and subradiant meta-atoms in a metamaterial structure. Han et al. have studied ultrafast, low-power, dynamically tunable slow light in an MDM waveguide coupled to cavity systems with nonlinear optical Kerr material.[24] The dynamic adjustment of the propagation phase of the plasmonic waveguide led to a pump light intensity of 11.7 MW/cm2 and a group index of up to 14.5. In addition, Zhu et al. have reported an all-optical PIT effect in metamaterials coated on ITO layers.[31] Hence, only a few studies have implemented ultrafast, low-power, dynamically adjustable PIT effects and slow light in plasmonic waveguide coupling systems through the dynamic adjustment of the frequency of the nanocavity and the propagation phase of the plasmonic waveguide.
Graphene is a single-layer carbon atom arranged in a bidimensional honeycomb lattice. The excellent electrical and optical properties of graphene endow this material a potential for application in photonic devices. Graphene has a large effective third-order nonlinear susceptibility χ(3) in the visible and near-infrared range, which has been validated through FWM[32] and Z-scan tests.[33] This distinct capability makes graphene a suitable material for the development of different tunable nanophotonic devices.[26] Therefore, the conventional nonlinear optical Kerr material is replaced with graphene to decrease the intensity of the pump light and to achieve low-power slow light in our study.
In this work, we investigate an ultrafast and low-power slow light tuning mechanism in PIT system through the dynamic adjustment of the frequency of the disk cavity and the propagation phase of the plasmonic waveguide. The simulation results indicate that when a single-layer graphene is used in the PIT system, the group velocity is controlled between c/53.2 and c/2.8 (c is the speed of light in vacuum). The numerical results show that the footprint of the PIT system is less than 0.8 μm2. Graphene can achieve response time in the order of 1 ps to tune an ultrafast response slow light. Thus, the provided ultracompact PIT structure has potential applications for slow light and dynamic light storage devices.
The rest of this paper is arranged as follows. Section
Figure
Figure
The Kerr nonlinear material is chosen as graphene in our work. Graphene films were grown on copper substrates by chemical vapor deposition (CVD) using methane in Ref. [34]. The dry transfer technique can be used to transfer graphene films onto the entire PIT system. First, relatively thick PMMA was coated on a graphene/copper foil. A polydimethylsiloxane (PDMS) block with a through hole in the center was attached to the PMMA/graphene/copper films by natural adhesion. The copper was then etched while the PDMS/PMMA/graphene block was floating over the solution. Using the PDMS “handle”, the composite was easily rinsed and dried after etching, thereby removing the liquid used in the etching process. Next, the PDMS/PMMA/graphene composite was placed onto the target substrate, covering the entire PIT system. The substrate was heated. The heat treatment allowed the wavy and rough PMMA/graphene film to make full contact with the target substrate. After heating, the adhesion of the graphene to the substrate was strong enough to peel off the PDMS block without delaminating the PMMA/graphene film. Finally, the PMMA was thermally removed in a furnace, without the use of any solvent. The graphene film was transferred onto the entire PIT system. At this time, the graphene film was covered on the entire PIT system. The graphene film that was covered on other areas except the areas of the upper part of the photonic device and the MDM plasmonic waveguide between the two disk resonators was etched by adopting inductively coupled plasma (ICP) etching process.[35] Hence, the graphene film was covered on the upper part of the photonic device (Fig.
The dynamic transmitted features of the plasmonic structure can be analyzed on the basis of coupled mode theory in accordance with frequency mistuning and phase shift between the two disk cavities. The dynamic formula of the cavity pattern amplitude yi of the i-th cavity (i = 1, 2) can be expressed as[36]
For simplicity, we suppose that only one incoming light (
The phase of the coupled factor is as assumed to be 0, which refers to θ1 = θ2 = 0. For the PIT system, the output transmitted efficiency can be calculated as
Electrical or optic modulation methods related to the heating effect have been used in many studies.[38,39] The modulation velocity of the heating effect is too low. In addition, the heating effects of nonlinear adsorption can interfere with the nonlinear dynamics if they are not correctly controlled. Numerous dynamic tuning mechanisms are available for photonic nonlinear devices, and these include slow light tuning with ultrafast response time and low pump power. An ultrafast response time can be achieved through optical Kerr modulation, and low pump power can be obtained by applying different nonlinear Kerr materials. Han et al. reported ultrafast, low-power, all-optical tunable PIT in an MDM waveguide side-coupled Fabry–Perot resonator system with a nonlinear organic polymer.[40] The intensity of the pump beam is high (i.e., usually about several gigawatts per square centimeter) because the third-order nonlinear susceptibility of organic polymers is small. The large pump power of the optical Kerr material restricts the use of integrated photonic devices.
Compared with the conventional Kerr nonlinear material, graphene has larger effective third-order Kerr coefficient. Gu et al. showed in experiments that graphene has a very high third-order nonlinear response.[41] Zhu et al. indicated that the linear refractive exponent of graphene is n0 = 2.4, and the large Kerr nonlinear coefficient is n2 = – 1.2 × 10−7 cm2/W, which is four orders of magnitude greater than that of nonlinear organic polymers.[26] The variation in the Kerr-induced refractive exponent is defined as Δ n = n2effI, where n2eff is the effective Kerr nonlinear coefficient and I is the pump light intensity. In this study, the graphene–Ag compound material structure has a large effective Kerr nonlinear coefficient of n2eff ≈ n2. The effective refractive exponent n of graphene is indicated as n = n0 + n2effI ≈ n0 + n2I.
In addition, Nikolaenko et al. demonstrated that an ultrafast response time of about 1 ps can be achieved in graphene.[42] Reckinger et al. also indicated that the resonant performance of plasmonic waveguide is affected by the refractive exponent of surrounding dielectric materials.[43] When a single-layer graphene is covered on the surface of a cavity or waveguide, the refractive exponent of the surrounding dielectric material varies. Such variation influences the resonant wavelength of the nanocavity and the phase shift of the plasmonic waveguide.
The total quality factor Qt of the disk cavity can be calculated from Qt = λ0/Δλ, where λ0 and Δλ are the peak wavelength and full width at half maximum of the reflection spectrum, respectively. If Qint ≫ Qc, the coupling quality factor can be calculated from the formula Qc = QintQt/(Qint – Qt). When the diameters of disk cavities 1 and 2 are set to 393 nm and 395 nm, respectively, Qint is about 530. The finite-difference time-domain (FDTD) simulation shows that Qt is approximately 65. Therefore, Qc is approximately 74.1. For the FDTD simulation, the time precision is set to 3000 fs and perfectly matched layer conditions are used to simulate. The steps of space and time are set to Δx = Δy = 2 nm and Δt = Δx/2c, respectively.
The frequency mistuning of the nanocavity is controlled by adjusting the resonant wavelength of the disk cavity. A pump beam with a wavelength of 830 nm is used. The FDTD simulation indicates that the resonant wavelength of disk cavity 2 is 788 nm. Disk cavity 1 is overlaid by a single-layer graphene. The effective refractive exponent of the graphene–Ag compound material structure is varied by using optical Kerr modulation. The resonant wavelength of disk cavity 1 is determined to λ = 40.65(n0 + Δn) + 690.44 nm via direct numerical modeling of the cavity.
The change in the resonance wavelength of the disk cavity under various pump light intensities when disk cavity 1 is overlaid by a single-layer graphene is shown in Fig.
Figure
Figures
This PIT system is considerably restrained by the delay–bandwidth product; the maximal accomplishable delay is conversely proportional to the operation bandwidth. That is, a tradeoff exists between frequency mistuning and group index. Hence, as indicated in Figs.
Figure
Figure
With the dispersion of the plasmonic waveguide, the cavity–cavity phase shift Δϕ1 can be expressed as Δϕ1 = ωs Re(neff)L/c, where ωs is the frequency of the signal light. neff is the effective refractive exponent and can be acquired by using the dispersion formula[36]
Figure
Details on the other structural parameters of the PIT systems are provided in this work. FDTD simulation shows that the resonant wavelengths of cavities 1 and 2 are 784 nm and 794 nm, respectively. The transparent wavelength is 789 nm.
The group index of PIT can be controlled by adjusting the propagation phase of the plasmonic waveguide with an 830 nm pump beam. In the dynamic situation, with optical Kerr effect, the effective refractive exponent variation causes the effective phase shift of the waveguide signal light Δϕ2 = 2π ΔneffL/λs, where Δneff is the variation of the effective refractive exponent caused by the Kerr effect, Δneff ≈ Δn, and λs is the wavelength of the signal light. In this work, when the pump light intensities are 5.88 MW/cm2 and 11.76 MW/cm2, the phase shifts of the signal light are 0.5π and π, respectively.
Thus, a portion of the phase shift between the two disk cavities stems from the dispersion of the SPPs wave in a static situation; the other portion is based on optical Kerr effect in the plasmonic waveguide in a dynamic situation. The unidirectional phase shift of the system (e.g., cavity–cavity phase shift) can be indicated as Δϕ = Δϕ1 + Δϕ2. The effective Kerr nonlinear coefficient of graphene is negative, and the phase shift of the signal light is reduced, which means Δϕ2 < 0. Cavity–cavity phase shift Δϕ can be tuned from π to 0 as the pump light intensity increases from 0 MW/cm2 to 11.76 MW/cm2 when Δϕ1 equals π.
Figure
Figures
The distributions of |Hz|2 are calculated at two dip wavelengths and at the transmitted peak wavelength via FDTD simulation to illustrate the physical cause of the PIT phenomenon. The results are presented in Figs.
Figure
An ultrafast and low-power slow light tuning mechanism based on the PIT effect in two disk cavities aperture-coupled to an MDM plasmonic waveguide system with a nonlinear optical Kerr material is investigated via theoretical and simulation methods. The group velocity is maintained between c/53.2 and c/15.1 with increasing pump light intensity from 0.41 MW/cm2 to 2.05 MW/cm2 by dynamic adjustment of the resonant frequency of the disk nanocavity via fine tuning of the group velocity. Meanwhile, the group velocity is maintained between c/2.8 and c/14.8 with increasing pump light intensity from 5.88 MW/cm2 to 11.76 MW/cm2; these can achieve a large tuning range of the group velocity by dynamic adjustment of the propagation phase of the plasmonic waveguide. The graphene–Ag compound material structure decreases the pump intensity because the local EM field of SPPs and slow light enhances the optical Kerr effect. Moreover, phase shift multiplication of the PIT effect is observed. The simulation results indicate that the entire structure is very compact, occupying less than 0.8μm2, and can achieve ultrafast response time in the order of 1 ps. The outcomes may pave the way for the design and fabrication of nanoscale supersensitive sensors, tunable slow-light devices, low-power optical storage, and ultrafast nonlinear devices in highly photonic integrated circuits.
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